Goodfellas - "layla" And reservoir dogs - "stick in the middle with you" are two that immediately come to mind. The opening credits song from Drive, Kavinsky's "Nightcall" is one of those just perfect combos that stuck with me. Also, an episode of Entourage used Radiohead's "fake plastic trees" in an awesome way as well. Entourage just used music in a great way all the time.
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