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The No Direction Home soundtrack has some great alternate and early takes on a number of classic Dylan songs, and some unreleased stuff too. I like the alternate version stuff the best. You might like it, it's two volumes.
The soundtrack to The Conversation is really good. It's very interesting, simple stuff. There is some elements of jazz, but it's mostly piano. There are two tracks that are annoying though, so skip those (they're loud and booming dark, for some horror scenes). Otherwise, great music.
Also, music from Ennio Morricone, including Once Upon a Time in the West/America and Good, Bad, Ugly.
And the music to A Beautiful Mind. Very mystical/operatic. I love it.
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